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Sign up to take. A Nature Research Journal. We demonstrate the bottom-up in-situ formation of organometallic oligomer chains at the single-molecule level. The chains are formed using the mechanically controllable break junction technique operated in a liquid environment, and consist of alternating isocyano-terminated benzene monomers coordinated to gold atoms.
We show that the chaining process is critically determined by the surface density of molecules. In particular, we demonstrate that by reducing the local supply of molecules within the junction, either by lowering the molecular concentration or by adding side groups, the oligomerization process can be suppressed.
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Their one-dimensional counterparts may offer alternative routes for bottom-up nanoscale electronics 7 aJime the ability of the transition metal Jqime to change oxidation states and greatly enhance their ability to transport charge 8.
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In-situ formation of one-dimensional coordination polymers in molecular junctions
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